Quantum science with ultracold molecules
Theo Murphy meeting organised by Professor Simon Cornish, Professor Michael Tarbutt and Dr Hannah Price.
Ultracold molecules offer a new and fascinating system for the study of many aspects of quantum science including ultracold chemistry, quantum computing, metrology, quantum simulation and fundamental physics. Following rapid recent progress, this meeting brought the community together to explore synergies with other disciplines and to map out the future avenues of research with ultracold molecules.
Attending this event
This meeting has taken place.
Enquiries: contact the Scientific Programmes team.
Organisers
Schedule
Chair
Hannah Price, Royal Society University Research Fellow and Proleptic Reader in Theoretical Physics, the University of Birmingham, UK
Hannah Price, Royal Society University Research Fellow and Proleptic Reader in Theoretical Physics, the University of Birmingham, UK
Hannah Price is a Royal Society University Research Fellow and a Proleptic Reader in Theoretical Physics at the University of Birmingham. Prior to arriving in Birmingham, she was a PhD student at the University of Cambridge and a postdoctoral researcher and Marie Skłodowska–Curie fellow at the INO-CNR BEC Center at the University of Trento, Italy. Her research group investigates the quantum simulation of topological phases of matter and quantum many-body states in platforms including ultracold atoms, molecules, photonics and mechanical systems.
09:00-09:05 |
Welcome by the lead organiser
|
---|---|
09:05-09:30 |
Measuring quantum correlations in a many-body system of polar molecules
Ultracold molecules have promising applications in the fields of quantum computing and simulation of many-body systems. Central to these applications is the ability to detect and manipulate the quantum state of individual molecules. Professor Bakr and his research group have recently developed a novel apparatus for imaging single diatomic molecules in an ultracold gas prepared in well-defined electronic, rovibrational and hyperfine states. Professor Bakr will describe how they used this capability to measure quantum correlations due to the quantum statistics of the molecules or due to entanglement mediated by dipolar interactions. As an example of a potential application, he will discuss their study of out-of-equilibrium dynamics in tunable quantum spin models and their measurements of the evolution of spatial correlations during the ensuing thermalization process. Professor Waseem Bakr, Princeton University, USA
Professor Waseem Bakr, Princeton University, USAProfessor Waseem Bakr is an associate professor of physics at Princeton University. He leads an experimental group focused on studying quantum many-body physics with ultracold gases of atoms and molecules. Professor Bakr obtained his PhD from Harvard University in 2011, where he developed the technique of quantum gas microscopy for detecting individual atoms in optical lattices and used it to perform microscopic studies of quantum phase transitions in bosonic lattice gases and quantum spin systems. He later extended the technique to fermionic atoms as a post-doc in the group of Martin Zwierlein at MIT. At Princeton, his group has used microscopy to study a variety of many-body phenomena in strongly-interacting lattice fermions, Rydberg-dressed ultracold gases and ultracold gases of polar molecules. |
09:30-09:45 |
Discussion
|
09:45-10:15 |
Synthetic dimensions in Rydberg atoms and dipolar molecules
The many accessible rotational states of molecules or electronic states of Rydberg atoms allow experiments to create synthetic dimensions, mimicking real-space motion by coupling of internal states. This provides extremely flexible engineering of single-particle physics, such as topological band structures, and when combined with dipolar interactions leads to rich physics. Professor Hazzard will describe a pair of recent experiments with Rydberg atom synthetic dimensions: a realisation of topological edge states (Killian & Dunning group, Nature Communications 13, 972 (2022)), and a first demonstration of interacting synthetic dimensions by using tweezer arrays, which is used to explore interacting particles in gauge fields (Gadway/Covey group, in preparation). He will discuss how interactions can lead to a wealth of novel phenomena: quantum strings/membranes, gapless symmetry-protected topological phases, or, dramatically. parastatistical quasiparticles, a type of particle beyond fermions and bosons. The author will conclude with the progress and rich opportunities for molecule synthetic dimensions. Professor Kaden Hazzard, Rice University, USA
Professor Kaden Hazzard, Rice University, USAKaden Hazzard is an Associate Professor at Rice University, where he studies how to understand and control quantum matter, especially in ultracold systems. He is interested in how to engineer increasingly complex or useful quantum states, and how to understand the rich behaviours that emerge in correlated quantum matter. He received his BS from Ohio State University and his PhD from Cornell University in 2010. He spent 2010-14 as a postdoc at JILA/CU-Boulder. Since July 2014, he has been faculty in the Rice University department of physics and astronomy. |
10:15-10:30 |
Discussion
|
10:30-11:00 |
Break
|
11:00-11:30 |
Tunable itinerant spin dynamics with dipolar molecules
Ultracold molecules enable exploration of exciting many-body physics due to their long-range, anisotropic dipolar interactions that govern dynamics in both internal and external degrees of freedom. Many scientific ideas based on this unique platform are now realizable due to recent experimental advances, including the production of quantum degenerate molecular gases, the shielding of inelastic collisions, the local state preparation and readout, and the precise tuning of a spin Hamiltonian. Annette Carroll will describe the recent study of tunable interactions between itinerant KRb molecules confined to 2D planes. At short times, the motion of the molecules is decoupled from the spin degree of freedom, and the spin dynamics are well-described by the mean field limit of the XXZ Hamiltonian. The mean field interaction, which shifts the rotational transition frequencies, was detected using Ramsey spectroscopy. The interaction’s strength and sign can be tuned with applied electric fields, as well as with the choice of rotational states. At longer times, elastic dipolar collisions, which couple the spin and motion, drive spin decoherence. This work paves the way for investigations of many-body spin-motion effects. Ms Annette Carroll, JILA, University of Colorado, USA
Ms Annette Carroll, JILA, University of Colorado, USAAnnette Carroll is a PhD student exploring many-body physics with dipolar molecules in Professor Jun Ye’s group at JILA. She received her bachelor’s degree from Princeton where she studied novel lattices for quantum simulation with Professor Andrew Houck. |
11:30-11:45 |
Discussion
|
11:45-12:15 |
Understanding and controlling collisions in quantum gases of NaK molecules
In this talk, Professor Ospelkaus will report about their recent experiments with quantum gases of polar bosonic 23Na39K molecules. She will first discuss inelastic atom-molecule and molecule-molecule collisions and their origin [1,2,3]. Afterwards she will discuss the control of atom-molecule collisions by Feshbach resonances as well as a proposal for blue shielding of collisions of polar molecules using optical photons at Raman resonance [4]. [1] Kai K. Voges, Philipp Gersema, Mara Meyer zum Alten Borgloh, Torben A. Schulze, Torsten Hartmann, Alessandro Zenesini, and Silke Ospelkaus (2020): Ultracold Gas of Bosonic 23Na39K Ground-State Molecules, Physical Review Letters 125, 083401 (2020) Professor Silke Ospelkaus, Leibniz University Hannover, Germany
Professor Silke Ospelkaus, Leibniz University Hannover, GermanySilke Ospelkaus studied physics at the University of Bonn and received her PhD in the field of ultracold atomic quantum gas mixtures from the University of Hamburg. With a Feodor Lynen Fellowship of the Alexander von Humboldt Foundation, she went to JILA, NIST and University of Colorado, USA as a postdoc in the group of Professor D Jin and Professor J Ye, where she worked on the preparation of ultracold molecular quantum gases from ultracold atomic quantum gas mixtures by means of a controlled chemical reaction. Subsequently, she was a Minerva group leader at the Max Planck Institute of Quantum Optics in the department of Professor I Bloch. Since 2011 she is Professor of Experimental Physics at Leibniz Universität Hannover, where she works on the preparation and control of molecular quantum gases. |
12:15-12:30 |
Discussion
|
12:30-13:30 |
Lunch
|
Chair
Professor Simon Cornish, Durham University, UK
Professor Simon Cornish, Durham University, UK
Simon L. Cornish is a Professor in the Department of Physics at Durham University working in the Quantum Light and Matter research group. He was educated at Oxford University where he received his PhD in experimental atomic physics in 1998. He developed an interest in ultracold gases at the University of Colorado, where he undertook pioneering experiments on Bose-Einstein condensation with tunable interactions. His current research focusses on the study of ultracold polar molecules formed by associating pairs of ultracold atoms, inspired by the prospect of using molecules as a platform for quantum simulation and quantum computation. He leads a national research program in the UK focused on the study of quantum science with ultracold molecules and was awarded the 2019 Institute of Physics Joseph Thomson medal and prize for outstanding contributions to experiments on ultracold atoms and molecules.
13:30-14:00 |
Optical tweezer arrays of laser-cooled molecules as a new platform for quantum science
Molecules, with their rich structure and tunable long-range interactions, have been proposed as a versatile platform for quantum science. In this talk, Professor Cheuk will report on recent advances from our group on controlling laser-cooled molecules that are trapped in optical tweezer arrays. He will describe their work on creating defect-free arrays of CaF molecules in 1D and observing coherent dipolar interactions between molecular pairs, and discuss how these results establish the building blocks for quantum information processing and quantum simulation of spin models using molecular tweezer arrays. Professor Cheuk will also report about their recent work towards full quantum control of laser-cooled molecules trapped in optical tweezers including their motional degrees of freedom. Specifically, he will report on Raman sideband cooling for molecules, and discuss how it provides a new pathway towards creating low-entropy molecular ensembles useful for quantum science. Professor Lawrence Cheuk, Princeton University, USA
Professor Lawrence Cheuk, Princeton University, USALawrence Cheuk received his Bachelor's degree in physics from Princeton University in 2010 and his PhD in atomic physics from MIT in 2017 focusing on quantum gas microscopy of strongly correlated fermionic systems. He subsequently moved to Harvard University as a Max-Planck/Harvard Quantum Optics postdoctoral fellow working on laser-cooled molecules. In 2020, he joined the physics faculty at Princeton University as an assistant professor. His current research interests lie in advancing control techniques for laser-cooled molecules and using molecules as a new platform for quantum science. He is an Alfred P. Sloan fellow and his research is supported by the NSF. |
---|---|
14:00-14:15 |
Discussion
|
14:15-14:45 |
Magic polarisation trapping of polar molecules for tunable dipolar interactions
Ultracold polar molecules can interact at long-range via electric dipole-dipole interactions, which can be controlled to entangle distant molecules by coherently coupling their rotational quantum states. Such capability, together with the abundance of rotational quantum states, makes polar molecules attractive for quantum simulation and computation. The author of the talk together with a group of researchers prepare an optical tweezer array of individual NaCs molecules in the ground state of their internal and motional degrees of freedom and perform rotational spectroscopy. In their system, the rotational coherence is predominantly limited by tweezer intensity noise, which induces differential light shifts between rotational states. To circumvent this problem, the researchers employ a new technique that uses 'magic' ellipticity trapping of polar molecules. With this technique, they reduce the differential polarisability by three orders of magnitude and improve the coherence time by an order of magnitude. With < 0.5 μm control over molecule position and site-selective rotational state control, the researchers expect to entangle the two adjacent rotational states within 1 ms. Dr Annie J Park, Harvard University, USA
Dr Annie J Park, Harvard University, USAAnnie J Park is a postdoctoral researcher in Professor Kang-Kuen Ni's group at Harvard University. Her research focuses on controlling ultracold polar molecules trapped in optical tweezers for quantum simulation and computation. Prior to joining the Ni group, she built a quantum simulator based on ultracold strontium atoms as a part of her PhD work in Professor Immanuel Bloch's group at the Max Planck Institute of Quantum Optics. |
14:45-15:00 |
Discussion
|
15:00-15:30 |
Break
|
15:30-16:00 |
Second-scale rotational coherence times in ultracold RbCs molecules
Ultracold polar molecules possess a rich network of rotational and hyperfine states that can be precisely coupled in experiments with resonant microwave fields. Engineering long-lived quantum coherences between rotational states is crucial for realising the full potential of ultracold molecules in current experiments. For molecules confined to optical traps, the rotational coherence time is typically limited by to the presence of large differential light shifts between the rotational states as a result of the anisotropic molecular polarisability. Here Dr Gregory will demonstrate a rotationally-magic optical trap for RbCs molecules that supports a Ramsey coherence time of 0.78(4) seconds, which extends to >1.4 seconds at the 95% confidence level using a single spin-echo pulse. In the researcher's magic trap, inhomogeneous and anisotropic dipolar interactions become the dominant source of decoherence, and they show that the coherence time is inversely proportional to the strength of these interactions. Dr Philip Gregory, Durham University, UK
Dr Philip Gregory, Durham University, UKPhilip Gregory is a post-doctoral research associate in the group of Simon Cornish at Durham University. During his PhD, he produced gases of ultracold RbCs molecules and developed techniques for coherent control of the rotational and hyperfine states of the molecules using resonant microwave fields. Since then, he has studied collisional processes between ultracold molecules revealing new insights into sticky collisions. Most recently, he has been focused on engineering long-lived rotational coherences in the molecules in order to observe effects from dipolar interactions in the bulk of gas of molecules. |
16:00-16:15 |
Discussion
|
16:15-16:45 |
Suppression of loss in ultracold NaRb molecules
In this presentation, Professor Wang will discuss their recent findings on mitigating the two-body loss of ground-state NaRb molecules. To achieve this, the scientists employ a blue-detuned microwave to create a long-range potential barrier, which significantly decreases the formation of the two-molecule complex, thereby reducing short-range loss by two orders of magnitude. Conversely, they observe a significant increase in elastic collisions, allowing the elastic collision rate to reach the hydrodynamic limit even at relatively low number densities. Additionally, the scientists demonstrate efficient evaporative cooling, but only within a specific density range. Professor Dajun Wang, the Chinese University of Hong Kong, China
Professor Dajun Wang, the Chinese University of Hong Kong, ChinaProfessor Dajun Wang obtained his PhD from the University of Connecticut in 2007. Before joining the Chinese University of Hong Kong, he worked as a postdoctoral research associate at JILA/University of Colorado from 2007 to 2010. His main research interests include ultracold polar molecules, ultracold chemical reaction, dipolar many-body physics, ultracold mixtures, and spinor systems. |
16:45-17:00 |
Discussion
|
17:00-18:15 |
Poster session
|
Chair
Professor Michael Tarbutt, Imperial College London, UK
Professor Michael Tarbutt, Imperial College London, UK
Mike Tarbutt is Professor of Experimental Physics at Imperial College London. He was educated at the University of Oxford where he received his PhD in 2001 for spectroscopic studies of highly charged ions. After postdoctoral work at the University of Sussex, he moved to Imperial and was awarded a University Research Fellowship from the Royal Society. He leads a research group focussed on laser-cooled molecules and their applications in quantum science and tests of fundamental physics. He is a Fellow of the American Physical Society and was awarded the 2022 Institute of Physics Joseph Thomson Medal and Prize.
12:15-12:30 |
Discussion
|
---|---|
09:00-09:30 |
Quantum simulation of the central spin model with a Rydberg atom and polar molecules in optical tweezers
Central spin models, where a single spinful particle interacts with a spin environment, find wide application in quantum information technology and can be used to describe, eg the decoherence of a qubit over time. The authors propose a method of realising an ultracold quantum simulator of a central spin model with XX (spin-exchanging) interactions [1]. The proposed system consists of a single Rydberg atom ("central spin") and surrounding polar molecules ("bath spins"), coupled to each other via dipole-dipole interactions. By mapping internal particle states to spin states, spin-exchanging interactions can be simulated. As an example system geometry, the authors consider a ring-shaped arrangement of bath spins, and show how it allows to exact precise control over the interaction strengths. They demonstrate that this setup allows to realise a central spin model with highly tunable parameters and geometry, for applications in quantum science and technology. [1] Dobrzyniecki J, Tomza, M 2023. ‘Quantum simulation of the central spin model with a Rydberg atom and polar molecules in optical tweezers,’arXiv:2302.14774v1 [quant-ph] Professor Michał Tomza, University of Warsaw, Poland
Professor Michał Tomza, University of Warsaw, PolandMichał Tomza is a university professor and head of the Quantum Molecular Systems research group and the Centre for Atomic Molecular and Optical Physics at the University of Warsaw. He specialises in the theory of interactions and collisions of ultracold atoms, ions, and molecules controlled with electromagnetic fields and their application in quantum science. He finished his PhD in quantum chemistry and theoretical physics in Warsaw, Poland, and in Kassel, Germany, in 2014. Next, he was a postdoctoral researcher in Vancouver, Canada, and in Barcelona, Spain. Since 2017, he has led his research group at the University of Warsaw. He has also conducted research as a visiting scientist at several institutions in Europe and the US. He has realised research grants awarded by the European Research Council (ERC) and Polish grant agencies. He is a member of the Polish Young Academy at the Polish Academy of Sciences. |
09:30-09:45 |
Discussion
|
09:45-10:15 |
Observation of Rydberg blockade due to the charge-dipole interaction between an atom and a polar molecule
Ultracold dipolar systems, including atoms excited to Rydberg states and polar molecules, hold great potential for quantum simulation and computation. Rydberg atoms offer strong, long-range interactions, which enable the engineering of quantum entanglement and multi-qubit gates through the Rydberg blockade mechanism. Polar molecules also exhibit long-range interactions and possess multiple long-lived rotational states that can be coupled using microwave fields to achieve high-fidelity quantum operations. Optical tweezer arrays have enabled the trapping of both these systems, creating the possibility of a hybrid system that combines the advantages of both platforms. This hybrid system offers new capabilities, including non-destructive readout of the molecular state, cooling of molecules using Rydberg atoms, and photoassociation of giant polyatomic Rydberg molecules. In this talk, Dr Guttridge will describe the first observation of Rydberg blockade due to the charge-dipole interaction between an atom and a polar molecule. The experiment involves the creation of a hybrid system consisting of ultracold RbCs molecules and Rb atoms trapped in species-specific optical tweezers. The researchers form weakly bound RbCs molecules by merging together optical tweezers containing Rb and Cs molecules. Strikingly, they find that weakly bound molecules can be produced without the widely used method of magnetoassociation across a Feshbach resonance but instead by exploiting an avoided crossing between atomic and molecular states as a function of tweezer separation. They transfer these weakly bound RbCs molecules to the rovibrational ground state using stimulated Raman adiabatic passage and achieve a one-way efficiency of 91(1)%. Finally, the researchers observe blockade of the transition to the Rb(52s) Rydberg state due to the charge-dipole interaction with a RbCs molecule in the rovibrational ground state. The blockade they have observed provides a mechanism for conditional and non-destructive state readout of the molecule and opens up many new research directions which Dr Guttridge will briefly discuss. Dr Alexander Guttridge, Durham University, UK
Dr Alexander Guttridge, Durham University, UKDr Alex Guttridge is a postdoctoral researcher at Durham University, whose research centres on quantum science with ultracold atoms and molecules. During his PhD, he produced the first ultracold mixtures of Cs and Yb atoms and studied their interactions through photoassociation spectroscopy of CsYb molecules. Currently, he leads a project that focusses on creating ultracold RbCs molecules in optical tweezers, which are formed from individually trapped Rb and Cs atoms. Recently, he has expanded his research to study hybrid systems of molecules and Rydberg atoms trapped in optical tweezer arrays, where he leads the investigation of this system as a researcher Co-I on the EPSRC funded project 'Interfacing Ultracold Polar Molecules with Rydberg atoms'. |
10:15-10:30 |
Discussion
|
10:30-11:00 |
Break
|
11:00-11:30 |
Quantum engineering of pair production process in spin models in multi- layers: from two- mode squeezing to topological Kitaev models
Understanding and controlling the growth and propagation of quantum correlations and entanglement is an emerging frontier in non-equilibrium many-body physics, and a crucial key step for unlocking the full advantage of quantum systems. In this talk Professor Ana Maria Rey will discuss how in multi-layer spin systems, currently accessible in a broad range of quantum platforms, such as arrays of neutral atoms, Rydberg atoms, magnetic atoms and polar molecules, spin interactions can be utilized to realize in a controllable manner a variety of correlated pair-production processes. In particular, the author will describe how in bi-layer systems, the capability to select individual layers and prepare targeted initial states, can enable the generation of iconic two-mode squeezing models that feature exponential growth of entanglement and are relevant in many contexts ranging from the foundations of quantum mechanics, to parametric amplification in quantum optics, to the Schwinger effect in high energy physics and Unruh thermal radiation in general relativity. In multi-layers the author will show it is possible to engineer a chiral bosonic Kitaev model featuring chiral propagation of correlations. Overall in this talk Professor Ana Maria Rey will report how current single layer addressing capabilities can allow shaping and controlling the temporal growth and spatial propagation of quantum correlations in a variety of spin systems relevant for quantum simulation. Dr Ana Maria Rey, JILA, NIST and University of Colorado Boulder, USA
Dr Ana Maria Rey, JILA, NIST and University of Colorado Boulder, USAAna Maria Rey obtained her bachelor’s degree in Physics in 1999 from the Universidad de los Andes in Bogota, Colombia. She pursued her graduate studies at the University of Maryland, College Park, receiving a PhD in 2004. She then joined the Institute of Theoretical, Molecular and Optical Physics at the Harvard-Smithsonian Center for Astrophysics as a Postdoctoral Fellow from 2005 to 2008. She joined JILA, NIST and the University of Colorado Boulder faculty in 2008. She is currently a JILA fellow and an associate research professor in the Department of Physics. Rey’s research focuses on how to control and manipulate ultra-cold atoms, molecules and trapped ions for use as quantum simulators of solid state materials and for quantum information and precision measurements. Rey’s recognition to her work include the APS Physics Outstanding Doctoral Thesis Award, the MacArthur Foundation Fellowship and the Presidential Early Career Award for Scientists and Engineers. |
11:30-11:45 |
Discussion
|
11:45-12:15 |
Degenerate Fermi gases of microwave-shielded polar molecules
Stable molecular Fermi gases with strong dipolar interactions provide unique opportunities for studying exotic quantum matter such as p-wave superfluidity and extended Fermi-Hubbard models. Dr Xin-Yu Luo will first show how they prepare a large degenerate Fermi gas of heteronuclear Feshbach molecules [1]. After being transferred to the rovibronic ground state, the scientists stabilize the molecular gas by microwave shielding while inducing strong elastic dipolar collisions. This enables the evaporation of polar molecules to temperatures well below the Fermi temperature [2]. The intermolecular potential can be flexibly tuned by the microwave field, allowing them to observe field-linked resonances in collisions of polar molecules. It provides a universal tuning knob to independently control the dipolar interaction and contact interaction [3]. In the end, Dr Xin-Yu Luo will discuss the perspective of realizing dipolar p-wave superfluidity in polar molecules [4] and their efforts towards further cooling down the molecular gas. [1] M. Duda et al, Transition from a polaronic condensate to a degenerate Fermi gas of heteronuclear molecules, Nature Physics 1-6 (2023) Dr Xin-Yu Luo, Max-Planck Institute for Quantum Optics, Germany
Dr Xin-Yu Luo, Max-Planck Institute for Quantum Optics, GermanyXin-Yu Luo obtained his PhD degree from the Institute of Physics, Chinese Academy of Science, in 2013. He has been a senior scientist leading the NaK molecules lab at the Max-Planck-Institute for Quantum Optics since 2018. He has been focusing on experiments of quantum manipulation and precision measurements with ultracold atoms and polar molecules. His current research interest is to understand and control the collisions of ultracold polar molecules and, subsequently, investigate strongly interacting dipolar quantum many-body systems. |
12:15-12:30 |
Discussion
|
Chair
Dr Hannah Williams, Durham University, UK
Dr Hannah Williams, Durham University, UK
Dr Williams completed her PhD at Imperial College London where she worked on the ultracold calcium fluoride (CaF) experiment. She achieved magneto-optical trapping and sub-Doppler cooling of CaF, as well as developing methods for coherent control over the internal quantum states of magnetically trapped molecules. Dr Williams then spent two years working in the group of Antoine Browaeys at the Institut d’Optique. Here her research focus changed to quantum simulation with Rydberg atoms and she demonstrated the Ising model on large 2d arrays of atoms and a Floquet pulse sequence for implementing the XXZ model. In October 2021, Dr Williams joined Durham University as an Assistant Professor where she is currently setting up a new experiment to investigated Zeeman -Sisyphus deceleration of molecules with the aim of building a quantum simulator using molecules.
13:30-14:00 |
Ultracold molecules for quantum science and particle physics
Polar molecules, due to their intrinsic electric dipole moment and their controllable complexity, are a powerful platform for precision measurement searches for physics beyond the standard model (BSM) and, potentially, for quantum simulation/computation. This has led to many experimental efforts to cool and control molecules at the single quantum state level, including with CaF. Professor Doyle will present work demonstrating entanglement and iSWAP operations with individual CaF molecules in optical tweezers. Polyatomic molecules have attracted new focus as potential novel quantum resources with distinct advantages - and challenges - compared to both atoms and diatomic molecules. He will discuss features of polyatomic molecules that can be used in quantum simulation/computation, the search for BSM physics, and ultracold chemistry. Professor Doyle will discuss the results on the laser cooling of polyatomic molecules into the ultracold regime, including the laser cooling of the polyatomic molecules SrOH, YbOH, CaOH and CaOCH3. Finally, if time permits, he will discuss recent measurements on spin precession in a metastable vibrational bending mode of CaOH, useful for future experiments searching for the electron electric dipole moment, a probe for BSM physics in the >10 TeV range. Professor John Doyle, Harvard University, USA
Professor John Doyle, Harvard University, USAJohn Doyle, Henry B Silsbee Professor of Physics, Harvard University, grew up in the US and received his bachelor’s (1986) and PhD (1991) degrees from the Massachusetts Institute of Technology (M.I.T.). After being a postdoc at M.I.T., he joined Harvard University as an assistant professor of physics in 1993. John Doyle's research centres on using cold molecules for science including particle physics, collisions, and quantum information. Starting with the development a new technique for producing heavy, polar radical molecules in an intense cold beam, he launched with collaborators searches for physics beyond the Standard Model (BSM) through probing for the electron electric dipole moment. His group is a pioneer in the cooling and trapping of molecules, studying collisional processes in atoms and molecules and developing tools to achieve full quantum control over increasingly complex molecular systems. They pioneered the laser cooling of polyatomic molecules and are working to realize new techniques to trap and study interactions in polyatomic molecules. John Doyle is the co-Director of the Harvard Quantum Initiative, director of the Japanese Undergraduate Research Exchange Program (JUREP), and he co-founded the Harvard/MIT Centre for Ultracold Atoms, where for twenty years he was co-director. He has published papers in the areas of ultracold atoms, molecules, spectroscopy, precision measurement, ultracold neutrons, respiratory disease transmission mitigation, and dark matter detection and supervised the PhDs of over thirty students. He is a Humboldt, Fulbright, and American Physical Society (APS) Fellow and a winner of the APS Broida prize and was elected president of the APS for 2025 (vice-president in 2023). |
---|---|
14:00-14:15 |
Discussion
|
14:15-14:45 |
Laser cooling of YO molecules to achieve high phase-space density
Ultracold molecules are a promising platform for precision physics, quantum chemistry, quantum simulation, and quantum information studies. In the last decade, there has been a flurry of interesting activity in the direct laser cooling of molecules, down to temperatures of a few μK. Recently, an optical tweezer array of molecules has been demonstrated. However, owing to the low phase-space density (PSD) of laser cooled polar molecules loaded into conservative traps, collisions in a bulk sample have remained elusive so far, in contrast to ultracold bialkali molecules created via association. Dr Aggarwal’s group is pursuing the goal of reaching quantum degeneracy of YO molecules. The PSD in conservative traps is limited largely by inefficient loading (few percent) due to large cloud sizes after sub-doppler cooling of molecules. In this talk, the author will present their recent results on the first sub-Doppler magneto-optical trap (MOT) of YO molecules [1]. The scientists observe volume compression by a factor of ~ 300 and temperature reduction by a factor of ~ 60 down to 30 μK in comparison to a conventional red detuned MOT, reaching a PSD several orders of magnitude higher than any previous molecular MOT. Currently, they are working on another cooling mechanism. YO has a low-lying excited state with a narrow transition linewidth of ~7 kHz. Optical photon scattering on this transition will result in cooling the molecules to recoil temperatures of 100s of nK. Dr Aggarwal will also present their progress so far on the narrow-line cooling of molecules. [1] Burau et al arXiv 2212.07472 (2022). Dr Parul Aggarwal, JILA, University of Colorado Boulder, USA
Dr Parul Aggarwal, JILA, University of Colorado Boulder, USADr Parul Aggarwal is a postdoctoral research associate working on the laser cooling and trapping of YO molecules in the group of Professor Jun Ye at JILA, University of Colorado Boulder, USA. She did her PhD work in the group of Professor Steven Hoekstra at the University of Groningen, the Netherlands. During her PhD, she worked on the production and Stark deceleration of molecular beams for an experiment aiming to make a precise measurement of an electron’s electric dipole moment. Dr Aggarwal did her Master’s research project on the study of Electromagnetically Induced Transparency in Rubidium atoms under the supervision of Professor Ajay Wasan at the Indian Institute of Technology Roorkee, India. |
14:45-15:00 |
Discussion
|
15:00-15:30 |
Break
|
15:30-16:00 |
Dipolar interactions of Rydberg atoms with polar molecules and superconducting circuits
The large electric dipole moments, ~ 1000 D, associated with transitions between high Rydberg states in atoms and molecules, offer opportunities to exploit resonant electric dipole interactions with polar ground state molecules, and with microwave fields in superconducting circuits for applications in quantum science. In this talk Professor Hogan will describe experiments in which resonant energy transfer, arising as a result of electric dipole-dipole interactions between helium Rydberg atoms and cold ground-state ammonia molecules, have been studied at temperatures below 100 mK and controlled using weak electric fields [1,2]. He will also describe experiments in which Rydberg atoms have been coherently coupled to microwave fields in superconducting co-planar waveguide resonators [3] in a setting that may open future opportunities for mediation of dipolar interactions with cold polar molecules over long range for applications in quantum simulation and information processing [4]. [1] K Gawlas and S D Hogan, J Phys Chem Lett 11, 83 (2020) Professor Stephen Hogan, University College London, UK
Professor Stephen Hogan, University College London, UKStephen Hogan is a professor of atomic and molecular physics and head of the Atomic Molecular Optical and Positron Physics group in the Department of Physics and Astronomy at University College London. He received his PhD in 2006 from Imperial College London and completed his Habilitation at ETH Zurich in 2012. His research interests centre around experiments with atoms and molecules in high Rydberg states. These include studies of resonant energy transfer in collisions of Rydberg atoms with polar molecules at low temperatures, investigations slow decay processes of cold electrostatically trapped Rydberg molecules, matter-wave interferometry with Rydberg atoms, the development of hybrid interfaces between Rydberg atoms and superconducting microwave circuits, and spectroscopy and tests of antimatter gravity with Rydberg positronium atoms. |
16:00-16:15 |
Discussion
|
16:15-17:00 |
Panel discussion/overview
Professor Simon Cornish, Durham University, UK
Professor Simon Cornish, Durham University, UKSimon L. Cornish is a Professor in the Department of Physics at Durham University working in the Quantum Light and Matter research group. He was educated at Oxford University where he received his PhD in experimental atomic physics in 1998. He developed an interest in ultracold gases at the University of Colorado, where he undertook pioneering experiments on Bose-Einstein condensation with tunable interactions. His current research focusses on the study of ultracold polar molecules formed by associating pairs of ultracold atoms, inspired by the prospect of using molecules as a platform for quantum simulation and quantum computation. He leads a national research program in the UK focused on the study of quantum science with ultracold molecules and was awarded the 2019 Institute of Physics Joseph Thomson medal and prize for outstanding contributions to experiments on ultracold atoms and molecules. Professor Lawrence Cheuk, Princeton University, USA
Professor Lawrence Cheuk, Princeton University, USALawrence Cheuk received his Bachelor's degree in physics from Princeton University in 2010 and his PhD in atomic physics from MIT in 2017 focusing on quantum gas microscopy of strongly correlated fermionic systems. He subsequently moved to Harvard University as a Max-Planck/Harvard Quantum Optics postdoctoral fellow working on laser-cooled molecules. In 2020, he joined the physics faculty at Princeton University as an assistant professor. His current research interests lie in advancing control techniques for laser-cooled molecules and using molecules as a new platform for quantum science. He is an Alfred P. Sloan fellow and his research is supported by the NSF. Dr Ana Maria Rey, JILA, NIST and University of Colorado Boulder, USA
Dr Ana Maria Rey, JILA, NIST and University of Colorado Boulder, USAAna Maria Rey obtained her bachelor’s degree in Physics in 1999 from the Universidad de los Andes in Bogota, Colombia. She pursued her graduate studies at the University of Maryland, College Park, receiving a PhD in 2004. She then joined the Institute of Theoretical, Molecular and Optical Physics at the Harvard-Smithsonian Center for Astrophysics as a Postdoctoral Fellow from 2005 to 2008. She joined JILA, NIST and the University of Colorado Boulder faculty in 2008. She is currently a JILA fellow and an associate research professor in the Department of Physics. Rey’s research focuses on how to control and manipulate ultra-cold atoms, molecules and trapped ions for use as quantum simulators of solid state materials and for quantum information and precision measurements. Rey’s recognition to her work include the APS Physics Outstanding Doctoral Thesis Award, the MacArthur Foundation Fellowship and the Presidential Early Career Award for Scientists and Engineers. Professor Silke Ospelkaus, Leibniz University Hannover, Germany
Professor Silke Ospelkaus, Leibniz University Hannover, GermanySilke Ospelkaus studied physics at the University of Bonn and received her PhD in the field of ultracold atomic quantum gas mixtures from the University of Hamburg. With a Feodor Lynen Fellowship of the Alexander von Humboldt Foundation, she went to JILA, NIST and University of Colorado, USA as a postdoc in the group of Professor D Jin and Professor J Ye, where she worked on the preparation of ultracold molecular quantum gases from ultracold atomic quantum gas mixtures by means of a controlled chemical reaction. Subsequently, she was a Minerva group leader at the Max Planck Institute of Quantum Optics in the department of Professor I Bloch. Since 2011 she is Professor of Experimental Physics at Leibniz Universität Hannover, where she works on the preparation and control of molecular quantum gases. Hannah Price, Royal Society University Research Fellow and Proleptic Reader in Theoretical Physics, the University of Birmingham, UK
Hannah Price, Royal Society University Research Fellow and Proleptic Reader in Theoretical Physics, the University of Birmingham, UKHannah Price is a Royal Society University Research Fellow and a Proleptic Reader in Theoretical Physics at the University of Birmingham. Prior to arriving in Birmingham, she was a PhD student at the University of Cambridge and a postdoctoral researcher and Marie Skłodowska–Curie fellow at the INO-CNR BEC Center at the University of Trento, Italy. Her research group investigates the quantum simulation of topological phases of matter and quantum many-body states in platforms including ultracold atoms, molecules, photonics and mechanical systems. Professor Michael Tarbutt, Imperial College London, UK
Professor Michael Tarbutt, Imperial College London, UKMike Tarbutt is Professor of Experimental Physics at Imperial College London. He was educated at the University of Oxford where he received his PhD in 2001 for spectroscopic studies of highly charged ions. After postdoctoral work at the University of Sussex, he moved to Imperial and was awarded a University Research Fellowship from the Royal Society. He leads a research group focussed on laser-cooled molecules and their applications in quantum science and tests of fundamental physics. He is a Fellow of the American Physical Society and was awarded the 2022 Institute of Physics Joseph Thomson Medal and Prize. |